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  1. Abstract Entropy dynamics is a Bayesian inference methodology that can be used to quantify time-dependent posterior probability densities that guide the development of complex material models using information theory. Here, we expand its application to non-Gaussian processes to evaluate how fractal structure can influence fractional hyperelasticity and viscoelasticity in elastomers. We investigate how kinematic constraints on fractal polymer network deformation influences the form of hyperelastic constitutive behavior and viscoelasticity in soft materials such as dielectric elastomers, which have applications in the development of adaptive structures. The modeling framework is validated on two dielectric elastomers, VHB 4910 and 4949, over a broad range of stretch rates. It is shown that local fractal time derivatives are equally effective at predicting viscoelasticity in these materials in comparison to nonlocal fractional time derivatives under constant stretch rates. We describe the origin of this accuracy that has implications for simulating large-scale problems such as finite element analysis given the differences in computational efficiency of nonlocal fractional derivatives versus local fractal derivatives. 
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    Free, publicly-accessible full text available August 1, 2024
  2. Auxetic foams exhibit novel mechanical properties due to their unique microstructure for improved energy-absorption and cavity expansion applications that have fascinated the scientific community since their inception. Given the advancements in material processing and performance of polymer open cell auxetic foams, there is a strong desire to fully understand the nonlinear rate-dependent deformation of these materials. The influence of nonlinear compressibility is introduced here along with relaxation effects to improve model predictions for different stretch rates and finite deformation regimes. The viscoelastic behavior of the material is analyzed by comparing fractional order and integer order calculus models. All results are statistically validated using maximum entropy methods to obtain Bayesian posterior densities for the hyperelastic, auxetic, and viscoelastic parameters. It is shown that fractional order viscoelasticity provides [Formula: see text]–[Formula: see text] improvement in prediction over integer order viscoelastic models when the model is calibrated at higher stretch rates where viscoelasticity is more significant.

     
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